Dokument: Drying of Soft Colloidal Films

Titel:Drying of Soft Colloidal Films
URL für Lesezeichen:https://docserv.uni-duesseldorf.de/servlets/DocumentServlet?id=68468
URN (NBN):urn:nbn:de:hbz:061-20250206-112558-3
Kollektion:Publikationen
Sprache:Englisch
Dokumententyp:Wissenschaftliche Texte » Artikel, Aufsatz
Medientyp:Text
Autoren: Kuk, Keumkyung [Autor]
Ringling, Julian [Autor]
Gräff, Kevin [Autor]
Hänsch, Sebastian [Autor]
Carrasco-Fadanelli, Virginia [Autor]
Rudov, Andrey A. [Autor]
Potemkin, Igor I. [Autor]
Klitzing, Regine von [Autor]
Buttinoni, Ivo [Autor]
Karg, Matthias [Autor]
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Dateien vom 06.02.2025 / geändert 06.02.2025
Stichwörter:fluid interface-mediated colloidal assembly, microgel-to-substrate adhesion, core-shell microgels, thin film, capillary forces
Beschreibung:Thin films made of deformable micro- and nano-units, such as biological membranes, polymer interfaces, and particle-laden liquid surfaces, exhibit a complex behavior during drying, with consequences for various applications like wound healing, coating technologies, and additive manufacturing. Studying the drying dynamics and structural changes of soft colloidal films
thus holds the potential to yield valuable insights to achieve improvements for applications. In this study, interfacial monolayers of core-shell (CS) microgels with varying degrees of softness are employed as model systems and to investigate their drying behavior on differently modified solid substrates (hydrophobic vs hydrophilic). By leveraging video microscopy,
particle tracking, and thin film interference, this study shed light on the interplay between microgel adhesion to solid surfaces and the immersion capillary forces that arise in the thin liquid film. It is discovered that a dried replica of the interfacial microstructure can be more accurately achieved on a hydrophobic substrate relative to a hydrophilic one, particularly when employing softer colloids as opposed to harder counterparts. These observations are qualitatively supported by experiments with a thin film
pressure balance which allows mimicking and controlling the drying process and by computer simulations with coarse-grained models.
Rechtliche Vermerke:Originalveröffentlichung:
Kuk, K., Ringling , J., Gräff, K., Hänsch, S., Carrasco Fadanelli, V., Rudov, A. A., Potemkin, I. I., von Klitzing, R., Buttinoni, I., & Karg, M. (2024). Drying of Soft Colloidal Films. Advanced Science, 11(47), Article 2406977. https://doi.org/10.1002/advs.202406977
Lizenz:Creative Commons Lizenzvertrag
Dieses Werk ist lizenziert unter einer Creative Commons Namensnennung 4.0 International Lizenz
Fachbereich / Einrichtung:Mathematisch- Naturwissenschaftliche Fakultät
Dokument erstellt am:06.02.2025
Dateien geändert am:06.02.2025
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